I had the exact same balance issues you described when I was hyperthyroid for years (had to suppress my TSH to 0.1 or below for thyroid cancer treatment). I doubt it's the Armour brand itself but rather your body adjusting to having a higher quantity of thyroid hormones in its system.
Six days of being on it is too soon to accurately check its impact with a TSH test, but definitely consult your doctor.
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